(with respect of course) I’d either disagree with the max 80V bit or suggest that maybe you’ve misunderstood. The 80V limit is recommended by Gecko as the max for their drives. They and Bob Campbell along with many others recommend that your motor voltage should be somewhere between 4 and 20 to 25 times the motors rated voltage. Your motors (at least your X and Y) you say are 2.7V so your power supply of 72V is 72/2.7 or 26.7 times, i.e. in excess of their recommendations. Maybe not by much but certainly on the high side. Also if I’m right in thinking your Z axis is a 2V motor then you’re at 36 times, well outside their recommendations.
Regarding "the higher the voltage, the faster the motors will go" - well... yes... in a way. What I think they meant is that the faster stepper motors go the less torque they produce. In order to keep the torque at a usable level at the highest speed you need, you usually need to up the voltage.
Sure, they're going to get slightly warm and I use that as my key to setting my voltages. My rule of thumb would be firstly set the current limiting resistors as advised by Gecko, then up the voltage until the motors run just warm over 15 minutes or so under load. If there's enough torque for the job at the max speed needed and V is below the 20 to 25 times the rated voltage then pay dirt. Otherwise the motors aren’t up to the job. I've read several times where it's said that they should be run hot, as in really hot. This I don't understand. To me, a hot motor is an inefficient and underpowered motor and wont last very long.
Oh yeah, my spindles (I have two rigs) are little Kress electronic 850s. Small I'm sure compared to some of the beasts out there but have proved big enough (just) for what I do at the moment.
Cheers
Stirling